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The electronic band structure of CoS2

Ning Wu1, Ya B Losovyj1,2, David Wisbey1, K Belashchenko1, M Manno3, L Wang3, C Leighton3 and P A Dowben1,4

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Angle-resolved and energy-dependent photoemission was used to study the band structure of paramagnetic CoS2 from high-quality single-crystal samples. A strongly dispersing hybridized Co–S band is identified along the Γ–X line. Fermi level crossings are also analysed along this line, and the results are interpreted using band structure calculations. The Fermi level crossings are very sensitive to the separation in the S–S dimer, and it is suggested that the half-metallic gap in CoS2 may be controlled by the bonding–antibonding splitting in this dimer, rather than by exchange splitting on the Co atoms.


PACS

71.20.-b Electron density of states and band structure of crystalline solids

79.60.-i Photoemission and photoelectron spectra

75.20.Ck Nonmetals

73.20.At Surface states, band structure, electron density of states

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Dates

Issue 15 (16 April 2007)

Received 9 January 2007, in final form 24 February 2007

Published 26 March 2007



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