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Formation of rodlike block copolymer micelles in aqueous salt solutions

V K Aswal1, A G Wagh1 and M Kammel2

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SANS measurements have been performed on the water-soluble PEO–PPO–PEO triblock copolymer P85 [(EO)26(PO)39(EO)26] in the presence of salts KCl, KF and K2CO3 in aqueous solution. Addition of these salts entropically favours dehydration from the micelles (similar to that of increasing temperature) and this leads to the formation of rodlike block copolymer micelles at ambient temperature. The rodlike micelles coexist with spherical micelles at higher salt concentrations or temperatures in these systems even up to the onset of phase separation. The hydration properties of the salt anions determine the population of the rodlike micelles.


PACS

61.25.H- Macromolecular and polymers solutions; polymer melts

82.70.Uv Surfactants, micellar solutions, vesicles, lamellae, amphiphilic systems, (hydrophilic and hydrophobic interactions)

61.05.fg Neutron scattering (including small-angle scattering)

Subjects

Soft matter, liquids and polymers

Chemical physics and physical chemistry

Dates

Issue 11 (21 March 2007)

Received 12 December 2006, in final form 20 January 2007

Published 27 February 2007



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