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Spin dynamics in Ho2Ru2O7

J S Gardner1,2, A L Cornelius3, L J Chang4,5, M Prager4, Th Brückel4 and G Ehlers6

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The spin relaxation processes within the pyrochlore Ho2Ru2O7 have been investigated by neutron scattering and bulk property techniques. A single-ion process, that is thermally activated, dominates the spin–spin relaxation spectrum above 2 K. Assuming Arrhenius behaviour, we found an activation energy Δ = (329 ± 6) K and characteristic relaxation time τ0 = (5.2 ± 0.3) × 10−12 s in the paramagnetic state, akin to those found in the spin ice, Ho2Ti2O7. Atlow temperature (T<95 K) the activation energy lowers and below 20 K the entropy and ac susceptibility are similar to that observed in other spin ice compounds within a 10 kOe field.


PACS

75.40.Gb Dynamic properties (dynamic susceptibility, spin waves, spin diffusion, dynamic scaling, etc.)

75.30.Cr Saturation moments and magnetic susceptibilities

61.05.fg Neutron scattering (including small-angle scattering)

Subjects

Condensed matter: electrical, magnetic and optical

Dates

Issue 44 (9 November 2005)

Received 18 August 2005, in final form 27 September 2005

Published 17 October 2005



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