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The coexistence of magnetic phases at the first-order phase transition of a metamagnet FeCl2centerdot2H2O studied by x-ray diffraction

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Y Narumi1,4, K Katsumata1, T Nakamura2, Y Tanaka1, S Shimomura3, T Ishikawa1 and M Yabashi2

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LETTER TO THE EDITOR

The results of non-resonant magnetic x-ray diffraction measurements of the metamagnet FeCl2centerdot2H2O subjected to an applied magnetic field, H, are reported. The material shows two successive first-order phase transitions: at Hc1 = 3.62 T from the antiferromagnetic (AF) to intermediate (I) phases, and at Hc2 = 4.67 T from phase I to a ferromagnetic phase at low temperatures. We find that the AF and I phases coexist over a wide range of H below Hc1, when H is decreased from the I phase. We were able to follow the evolution of the AF and I domains with the change of H. The coexistence appears not to come from demagnetizing effects, and instead reflects the intrinsic nature of the material.


PACS

75.30.Kz Magnetic phase boundaries (including magnetic transitions, metamagnetism, etc.)

75.40.Cx Static properties (order parameter, static susceptibility, heat capacities, critical exponents, etc.)

75.60.Ch Domain walls and domain structure

75.50.-y Studies of specific magnetic materials

Subjects

Condensed matter: electrical, magnetic and optical

Dates

Issue 7 (25 February 2004)

Received 13 November 2003

Published 6 February 2004



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