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Scaling in soft spheres: fragility invariance on the repulsive potential softness

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Cristiano De Michele1,2, Francesco Sciortino1 and Antonio Coniglio2

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LETTER TO THE EDITOR

We address the question of the dependence of the fragility of glass forming supercooled liquids on the 'softness' of an interacting potential by performing numerical simulation of a binary mixture of soft spheres with different power n of the interparticle repulsive potential. We show that the temperature dependence of the diffusion coefficients for various n collapses onto a universal curve, supporting the unexpected view that fragility is not related to the hard core repulsion. We also find that the configurational entropy correlates with the slowing down of the dynamics for all studied n.


PACS

65.60.+a Thermal properties of amorphous solids and glasses: heat capacity, thermal expansion, etc.

66.30.-h Diffusion in solids

64.70.P- Glass transitions of specific systems

Subjects

Condensed matter: structural, mechanical & thermal

Dates

Issue 45 (17 November 2004)

Received 14 September 2004

Published 29 October 2004



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