Quick search Find article
Quick search
Find article

The crystal structure and electronic properties of a new metastable non-stoichiometric BaAl4-type compound crystallized from amorphous La6Ni34Ge60 alloy

Masashi Hasegawa1, Shoichiro Suzuki1, Tetsu Ohsuna1, Eiichiro Matsubara1, Satoshi Endo2 and Akihisa Inoue1

Show affiliations


A new metastable La–Ge–Ni ternary BaAl4-type (ThCr2Si2-type) compound, of which the space group is I4/mmm is synthesized. It is obtained by a polymorphic transformation from an La6Ni34Ge60 amorphous alloy on crystallizing. The formula of the compound is (La0.3Ge0.7)(Ni0.85Ge0.15)2Ge2. This indicates that it is highly non-stoichiometric compared to the stoichiometric LaNi2Ge2. It is found that the c-axis lattice parameter of this compound is much longer than that of LaNi2Ge2. It should be noted that the longer c-axis unit cell parameter is attributable only to the longer interlayer distance between Ge site and Ni site layers. The temperature dependences of electrical resistivity and thermoelectric power of the (La0.3Ge0.7)(Ni0.85Ge0.15)2Ge2 compound and La6Ni34Ge60 amorphous alloy are also clarified. The comparison of these electronic properties between the two materials indicates that sp-electrons mainly contribute to the density of states around the Fermi level of this compound.


PACS

61.66.Fn Inorganic compounds

72.20.Pa Thermoelectric and thermomagnetic effects

61.66.Dk Alloys

72.15.Eb Electrical and thermal conduction in crystalline metals and alloys

72.80.Jc Other crystalline inorganic semiconductors

61.50.Ks Crystallographic aspects of phase transformations; pressure effects

72.15.Jf Thermoelectric and thermomagnetic effects

Subjects

Condensed matter: electrical, magnetic and optical

Semiconductors

Condensed matter: structural, mechanical & thermal

Dates

Issue 45 (17 November 2004)

Received 28 July 2004, in final form 10 September 2004

Published 29 October 2004



  1. The crystal structure and electronic properties of a new metastable non-stoichiometric BaAl4-type compound crystallized from amorphous La6Ni34Ge60 alloy

    Masashi Hasegawa et al 2004 J. Phys.: Condens. Matter 16 7917

  2. Young's double-slit experiment using core-level photoemission from N2: revisiting Cohen–Fano's two-centre interference phenomenon

    X-J Liu et al 2006 J. Phys. B: At. Mol. Opt. Phys. 39 4801

  3. Quadrupole collective variables in the natural Cartan–Weyl basis

    S De Baerdemacker et al 2007 J. Phys. A: Math. Theor. 40 2733

  4. A canonical approach to the quantization of the damped harmonic oscillator

    Rabin Banerjee and Pradip Mukherjee 2002 J. Phys. A: Math. Gen. 35 5591

  5. Photoionization-Driven X-Ray Line Emission in Cygnus X-3

    Duane A. Liedahl and Frits Paerels 1996 ApJ 468 L33

  6. The diamagnetic Coulomb problem: an eigenvalue problem with two singularities

    S Barcza 2005 J. Phys. A: Math. Gen. 38 2469

  7. Properties of the solvation force of a two-dimensional Ising strip in scaling regimes

    Piotr Nowakowski and Marek Napiórkowski 2009 J. Phys. A: Math. Theor. 42 475005

  8. Optical and acoustic properties at 1064 nm of polyvinyl chloride-plastisol for use as a tissue phantom in biomedical optoacoustics

    Gloria M Spirou et al 2005 Phys. Med. Biol. 50 N141

  9. The Coronae of Moderate-Mass Giants in the Hertzsprung Gap and the Clump

    Thomas R. Ayres et al. 1998 ApJ 496 428

  10. Arc attachment and fall voltage on the cathode of an ac high-pressure mercury discharge

    H Pursch et al 2002 J. Phys. D: Appl. Phys. 35 1757

Related review articles

What's this?
View review articles related to this research to gain an insight into the key trends in this subject area. Related review articles are selected based on PACS/MSC codes, and are no more than three years old.

  1. Magnesium dititanate (MgTi2O5) with pseudobrookite structure: a review
  2. Structure of silicon/oxide and nitride/oxide interfaces

View by subject




Export








Please login to access our web services, or create an account if you don't yet have one.

You must have cookies enabled in your web browser to be able to login.

Username
Password

Forgotten your password? Get a new one here.