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Conduction bands in the filled skutterudites

Hisatomo Harima1 and Katsuhiko Takegahara2

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Some filled skutterudite compounds have recently been found to exhibit very interesting properties: a metal–insulator transition (PrRu4P12), an antiferroquadrupole ordering and heavy-fermion behaviour under magnetic fields (PrFe4P12) and a new class of heavy-fermion superconductivity (PrOs4Sb12). Such varied and interesting physical properties are thought to reflect the Fermi surface properties. Band structure calculations have revealed the characteristics of the conduction bands. The main conduction band consisting of p orbitals of pnictogen surrounding the rare-earth ions has a nesting property, and strongly hybridizes with one of 4f electrons. One of the other conduction bands does not have mixing matrix elements with 4f electrons, resulting in the unique band structure in CeOs4Sb12.


PACS

71.20.Eh Rare earth metals and alloys

71.27.+a Strongly correlated electron systems; heavy fermions

73.20.At Surface states, band structure, electron density of states

71.30.+h Metal-insulator transitions and other electronic transitions

71.18.+y Fermi surface: calculations and measurements; effective mass, g factor

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Dates

Issue 28 (23 July 2003)

Received 12 November 2002

Published 4 July 2003



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