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Curvature and strain effects on electronic properties of single-wall carbon nanotubes

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J W Ding1,2, X H Yan1, J X Cao1,2, D L Wang1,2, Y Tang1 and Q B Yang1

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LETTER TO THE EDITOR

To describe accurately the electronic structures of carbon nanotubes, a semi-empirical tight-binding approach is presented in which the main intrinsic curvatures have been fully taken into account. The calculated electronic structures and band gaps are consistent with experimental measurements. Studies of the relative importance of various intrinsic curvatures show that each curvature has a contribution of varying importance to the curvature-induced band gap. Additionally, under both uniaxial and torsional strain, semiconductor–metal–semiconductor phase transitions have been observed for primary metallic carbon nanotubes. The critical stress of the transition and the gap's sensitivity with stress are dependent on both the diameter and chirality of nanotubes, which is at variance with previous predictions.


PACS

62.25.-g Mechanical properties of nanoscale systems

71.15.Ap Basis sets (LCAO, plane-wave, APW, etc.) and related methodology (scattering methods, ASA, linearized methods, etc.)

73.22.-f Electronic structure of nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals

Subjects

Condensed matter: electrical, magnetic and optical

Nanoscale science and low-D systems

Dates

Issue 27 (16 July 2003)

Received 23 May 2003

Published 27 June 2003



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