Quick search Find article
Quick search
Find article

Looking for the glass transition in a single molecular layer on the water surface

L Cristofolini1, P Cicuta2 and M P Fontana1

Show affiliations


We present here results which indicate that polymeric monolayers confined at the air–water interface may provide interesting model systems for the study of glass transition phenomenology in a strongly confined 2D geometry. We report on photoinduced relaxation of the pressure–area isotherms in Langmuir monolayers of a photosensitive polyacrylate, using null-ellipsometry to study the evolution of the film thickness in the neighbourhood of the bulk glass transition. Furthermore, viscoelastic behaviour is investigated by a combination of surface quasielastic light scattering and expansion–compression isothermal cycles.


PACS

64.70.P- Glass transitions of specific systems

61.41.+e Polymers, elastomers, and plastics

68.03.-g Gas-liquid and vacuum-liquid interfaces

62.40.+i Anelasticity, internal friction, stress relaxation, and mechanical resonances

68.18.Jk Phase transitions in liquid thin films

78.68.+m Optical properties of surfaces

Subjects

Soft matter, liquids and polymers

Surfaces, interfaces and thin films

Condensed matter: structural, mechanical & thermal

Dates

Issue 11 (26 March 2003)

Received 27 September 2002

Published 10 March 2003



  1. Looking for the glass transition in a single molecular layer on the water surface

    L Cristofolini et al 2003 J. Phys.: Condens. Matter 15 S1031

  2. Influence of Cd impurity on the electronic properties of CuAlO2 delafossite: first-principles calculations

    M V Lalic et al 2002 J. Phys.: Condens. Matter 14 5517

  3. Friction experiments on the nanometre scale

    E Gnecco et al 2001 J. Phys.: Condens. Matter 13 R619

  4. The absence of finite-temperature phase transitions in low-dimensional many-body models: a survey and new results

    Axel Gelfert and Wolfgang Nolting 2001 J. Phys.: Condens. Matter 13 R505

  5. Lifetime measurements in Ru II and calculated oscillator strengths in Ru II and Ru III

    P Palmeri et al 2009 J. Phys. B: At. Mol. Opt. Phys. 42 165005

  6. Calorimetry of Bose–Einstein condensates

    P B Blakie et al 2007 J. Phys. B: At. Mol. Opt. Phys. 40 3273

  7. Mechanisms of cluster ionization in strong laser pulses

    U Saalmann et al 2006 J. Phys. B: At. Mol. Opt. Phys. 39 R39

  8. Partial photoionization cross sections of doubly excited helium below the ionization thresholds I8 and I9

    Y H Jiang et al 2006 J. Phys. B: At. Mol. Opt. Phys. 39 L9

  9. Cold atom clocks and applications

    S Bize et al 2005 J. Phys. B: At. Mol. Opt. Phys. 38 S449

  10. Spontaneous-emission suppression via multiphoton quantum interference

    Jörg Evers and Christoph H Keitel 2004 J. Phys. B: At. Mol. Opt. Phys. 37 2771

Related review articles

What's this?
View review articles related to this research to gain an insight into the key trends in this subject area. Related review articles are selected based on PACS/MSC codes, and are no more than three years old.

  1. Photoinduced phase transitions
  2. Evolution of the structure of amorphous alloys
  3. Processes involving clusters and small particles in a buffer gas
More

View by subject




Export








Please login to access our web services, or create an account if you don't yet have one.

You must have cookies enabled in your web browser to be able to login.

Username
Password

Forgotten your password? Get a new one here.