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Pressure effects on first-order magnetic Raman scattering in NiO

Y Mita1, Y Ishida1, M Kobayashi1,2 and S Endo2,3

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The pressure dependence of first-order magnetic Raman peak of NiO single crystal was studied up to 20 GPa at room temperature. At ambient pressure, an unknown peak is also observed at nearly the same position as the one-magnon one and their separation becomes remarkable with increasing pressure. Pressure coefficients of the one-magnon peak and the other peak are obtained as 0.4 and 1.5 cm−1 GPa−1, respectively. The next-nearest-neighbour antiferromagnetic exchange constant J2 is obtained as a function of the lattice constant.


PACS

78.30.Hv Other nonmetallic inorganics

61.66.Fn Inorganic compounds

75.30.Et Exchange and superexchange interactions

75.50.Ee Antiferromagnetics

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 44 (11 November 2002)

Received 25 June 2002

Published 25 October 2002



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