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A new macroscopically degenerate ground state in the spin ice compound Dy2Ti2O7 under a magnetic field

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K Matsuhira1, Z Hiroi2, T Tayama2, S Takagi1 and T Sakakibara2

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LETTER TO THE EDITOR

The low-temperature magnetic properties of the pyrochlore compound Dy2Ti2O7 in magnetic fields applied along the [111] direction are reported. Below 1 K, a clear plateau has been observed in the magnetization process in the field range 2–9 kOe, followed by a sharp moment jump at around 10 kOe that corresponds to a breaking of the spin ice state. We found that the plateau state is disordered, with a residual entropy of nearly half the value for the zero-field state, whose macroscopic degeneracy comes from a frustration of the spins on the Kagomé layers perpendicular to the magnetic field.


PACS

75.60.Ej Magnetization curves, hysteresis, Barkhausen and related effects

75.40.-s Critical-point effects, specific heats, short-range order

65.40.G- Other thermodynamical quantities

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 29 (29 July 2002)

Received 7 June 2002

Published 11 July 2002



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