N Stüßer et al 2002 J. Phys.: Condens. Matter 14 5161 doi:10.1088/0953-8984/14/20/311
N Stüßer1, U Schotte1, A Hoser1,2, M Meschke1, M Meißner1 and J Wosnitza3
Show affiliationsNeutron diffraction investigations have been performed to study the magnetization process of CsCuCl3 with the magnetic field aligned within the ab-plane. In zero field the stacked, triangular-lattice antiferromagnet (TLA) CsCuCl3 has a helical structure incommensurate in the chain direction normal to the ab-plane. The magnetic phase diagram was investigated from 2 K up to TN in fields up to 17 T. The phase line for the expected incommensurate-commensurate (IC-C) phase transition could be determined throughout the whole phase diagram. At low temperature the IC-C transition is roughly at half the saturation field HS. The neutron diffraction patterns were found to be well described by a sinusoidally modulated spiral in fields up to HS/3. The initial increase of the scattering intensity in rising field indicates a continuous reduction of the spin frustration on the triangular lattice. Between HS/3 and HS/2 a new phase occurs where the spiral vector has a plateau in its field dependence. Close to the IC-C transition a growing asymmetry of magnetic satellite-peak intensities indicates domain effects which are related to the lifting of the chiral degeneracy in the ab-plane in rising field. The phase diagram obtained has some similarities with those calculated for stacked TLAs by considering the effects of quantum and thermal fluctuations.
64.70.Rh Commensurate-incommensurate transitions
75.30.Sg Magnetocaloric effect, magnetic cooling
75.60.Ej Magnetization curves, hysteresis, Barkhausen and related effects
75.30.Kz Magnetic phase boundaries (including magnetic transitions, metamagnetism, etc.)
Issue 20 (27 May 2002)
Received 5 February 2002, in final form 11 April 2002
Published 9 May 2002
N Stüßer et al 2002 J. Phys.: Condens. Matter 14 5161
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