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A neutron diffraction study of the magnetic phases of CsCuCl3 for in-plane fields up to 17 T

N Stüßer1, U Schotte1, A Hoser1,2, M Meschke1, M Meißner1 and J Wosnitza3

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Neutron diffraction investigations have been performed to study the magnetization process of CsCuCl3 with the magnetic field aligned within the ab-plane. In zero field the stacked, triangular-lattice antiferromagnet (TLA) CsCuCl3 has a helical structure incommensurate in the chain direction normal to the ab-plane. The magnetic phase diagram was investigated from 2 K up to TN in fields up to 17 T. The phase line for the expected incommensurate-commensurate (IC-C) phase transition could be determined throughout the whole phase diagram. At low temperature the IC-C transition is roughly at half the saturation field HS. The neutron diffraction patterns were found to be well described by a sinusoidally modulated spiral in fields up to HS/3. The initial increase of the scattering intensity in rising field indicates a continuous reduction of the spin frustration on the triangular lattice. Between HS/3 and HS/2 a new phase occurs where the spiral vector has a plateau in its field dependence. Close to the IC-C transition a growing asymmetry of magnetic satellite-peak intensities indicates domain effects which are related to the lifting of the chiral degeneracy in the ab-plane in rising field. The phase diagram obtained has some similarities with those calculated for stacked TLAs by considering the effects of quantum and thermal fluctuations.


PACS

61.05.fm Neutron diffraction

64.70.Rh Commensurate-incommensurate transitions

75.30.Sg Magnetocaloric effect, magnetic cooling

75.60.Ej Magnetization curves, hysteresis, Barkhausen and related effects

75.30.Kz Magnetic phase boundaries (including magnetic transitions, metamagnetism, etc.)

75.50.Ee Antiferromagnetics

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 20 (27 May 2002)

Received 5 February 2002, in final form 11 April 2002

Published 9 May 2002



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