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Variation of adatom to substrate charge transfer value along the first-row transition metal series on Mo(110)

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T T Magkoev1,4, K Christmann2, P Lecante3,5 and A M C Moutinho3

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LETTER TO THE EDITOR

Adsorption of the first-row transition 3d metals (Ti-Cu) on the atomically clean Mo(110) surface in ultra-high-vacuum conditions has been studied by Auger electron spectroscopy and work function measurements (Anderson method). In this letter it is shown that adsorption behaviour of the metals under consideration systematically changes along the 3d series. The observed correlation between the systematic change of the dipole moments and the values of the charge transfer from adatom to substrate along the period leads us to the conclusion that the metal 3d orbitals play an important role in the formation of the chemisorption bond.


PACS

68.43.Mn Adsorption kinetics

68.49.Jk Electron scattering from surfaces

73.30.+y Surface double layers, Schottky barriers, and work functions

79.20.Fv Electron impact: Auger emission

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Dates

Issue 12 (1 April 2002)

Received 14 December 2001

Published 15 March 2002



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