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Magnetic and transport properties of a new valence-fluctuating compound, CeRhP

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T Sasakawa, T Suemitsu, J Kitagawa, O Sologub, P Salamakha and T Takabatake1

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LETTER TO THE EDITOR

We have synthesized CeRhP, aiming at breaking new ground as regards the CeRhPn (Pn = pnictogen) system. X-ray powder diffraction analysis shows that CeRhP crystallizes into the tetragonal LaPtSi-type structure. Both the magnetic susceptibility and thermopower exhibit a broad peak around 170 K, and the specific heat gives an electronic specific-heat coefficient of 30 mJ K-2 mol-1. These results indicate that CeRhP is a valence-fluctuating compound with a Kondo temperature of 400-500 K. The electrical resistivity shows a metallic behaviour, in contrast to the semimetal or semiconducting behaviour in CeRhSb and CeRhAs, with the orthorhombic ε-TiNiSi-type structure. This stresses the importance of the crystal symmetry to the gap formation in the CeRhPn series.


PACS

75.30.Cr Saturation moments and magnetic susceptibilities

75.40.Cx Static properties (order parameter, static susceptibility, heat capacities, critical exponents, etc.)

61.66.Fn Inorganic compounds

61.50.Ah Theory of crystal structure, crystal symmetry; calculations and modeling

72.15.Jf Thermoelectric and thermomagnetic effects

75.30.Mb Valence fluctuation, Kondo lattice, and heavy-fermion phenomena

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 12 (1 April 2002)

Received 6 February 2002, in final form 19 February 2002

Published 15 March 2002



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