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Magnetization density distribution in

J A Paixão-+, L C J Pereira++, P Estrela§, M Godinho§, M Almeida-+, L Paolasini||, M Bonnet, J Rebizant+ and J C Spirlet+

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A magnetization density study by means of polarized-neutron scattering on the intermetallic compound is reported. belongs to the large (An = U, Np, Pu, Am; T = transition metal; X = In, Sn) family of compounds crystallizing in an ordered variant of the tetragonal type of structure (space group ). does not order magnetically but has a large magnetic susceptibility that qualifies it as an enhanced paramagnet or spin fluctuator. We report single-crystal magnetization measurements that show a significant magnetic anisotropy, with a c-axis susceptibility exceeding that measured on the basal plane by a factor of four. The magnetization density distribution in the unit cell was measured at 2 K by polarized-neutron scattering under a magnetic field of 5.5 T applied parallel to the c-axis. It was found that the major contribution to the magnetic susceptibility is located on the U atoms but a small response from the Co atoms is also measured .


PACS

75.60.Ej Magnetization curves, hysteresis, Barkhausen and related effects

75.30.Cr Saturation moments and magnetic susceptibilities

61.66.Dk Alloys

75.30.Gw Magnetic anisotropy

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 9 (8 March 1999)

Received 27 August 1998



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