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Angle dependence of the upper critical field in the layered organic superconductor kappa-(BEDT-TTF)2Cu(NCS)2 (BEDT-TTFequiv bis(ethylene-dithio)tetrathiafulvalene)

M-S Nam-+, J A Symington-+, J Singleton-+, S J Blundell-+, A Ardavan-+, J A A J Perenboom++, M Kurmoo§ and P Day||

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LETTER TO THE EDITOR

We have performed detailed studies of the angle- and temperature-dependent resistive upper critical fields in the layered organic superconductor kappa-(BEDT-TTF)2Cu(NCS)2. With the magnetic field lying in the conducting planes, our measurements show an upper critical field which comfortably exceeds the Pauli-paramagnetic limit in this material. We find no azimuthal angle dependence of the critical field, in spite of recent evidence that this material has gap nodes characteristic of d-wave superconductivity. We propose that the large critical fields may be due to a Fulde-Ferrell-Larkin-Ovchinnikov state which can exist in exactly in-plane fields because of the nature of the Fermi surface of kappa-(BEDT-TTF)2Cu(NCS)2.


PACS

74.70.Kn Organic superconductors

74.20.Rp Pairing symmetries (other than s-wave)

74.25.Op Mixed states, critical fields, and surface sheaths

74.25.Ha Magnetic properties

Subjects

Superconductivity

Dates

Issue 43 (1 November 1999)

Received 15 July 1999



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