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Generation of broad XUV continuous high harmonic spectra and isolated attosecond pulses with intense mid-infrared lasers

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C Trallero-Herrero1,2, Cheng Jin1, B E Schmidt3, A D Shiner2, J-C Kieffer3, P B Corkum2, D M Villeneuve2, C D Lin1, F Légaré3 and A T Le1

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We present experimental results showing the appearance of a near-continuum in the high-order harmonic generation spectra of atomic and molecular species as the driving laser intensity of a mid-infrared pulse increases. Detailed macroscopic simulations reveal that these near-continuum spectra are capable of producing isolated attosecond pulses (IAPs) in the far field if a proper spatial filter is applied. Further, our simulations show that the near-continuum spectra and the IAPs are a product of the strong temporal and spatial reshaping (blue shift and defocusing) of the driving field. This offers a possibility of producing IAPs with a broad range of photon energy, including plateau harmonics, by mid-IR laser pulses even without carrier-envelope phase stabilization.


PACS

42.65.Ky Frequency conversion; harmonic generation, including higher-order harmonic generation

32.30.Jc Visible and ultraviolet spectra

33.70.Jg Line and band widths, shapes, and shifts

32.70.Jz Line shapes, widths, and shifts

32.80.Fb Photoionization of atoms and ions

33.80.Eh Autoionization, photoionization, and photodetachment

Subjects

Atomic and molecular physics

Optics, quantum optics and lasers

Dates

Issue 1 (14 January 2012)

Received 5 October 2011, in final form 5 November 2011

Published 9 December 2011



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