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Term-dependent lifetime broadening effect on the 4d photoelectron spectrum of atomic thulium

A G Kochur1, I D Petrov1, J Schulz2 and Ph Wernet3

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The 4d photoelectron spectrum of free thulium atoms is measured and calculated in the single-configuration intermediate-coupling approximation considering multiplet splitting and lifetime broadening of the spectral components due to radiationless transitions following the 4d ionization. The individual natural widths of the 4d94f13 multiplet components are found to differ considerably, and the experimental profile of the spectrum can be reproduced theoretically only if this effect is taken into account.


PACS

32.80.Fb Photoionization of atoms and ions

32.50.+d Fluorescence, phosphorescence (including quenching)

32.70.Jz Line shapes, widths, and shifts

Subjects

Atomic and molecular physics

Dates

Issue 21 (14 November 2008)

Received 24 July 2008, in final form 16 September 2008

Published 23 October 2008



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