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Pump–probe experiments in atoms involving laser and synchrotron radiation: an overview

REVIEW ARTICLE

F J Wuilleumier and M Meyer

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TOPICAL REVIEW

The combined use of laser and synchrotron radiations for atomic photoionization studies started in the early 1980s. The strong potential of these pump–probe experiments to gain information on excited atomic states is illustrated through some exemplary studies. The first series of experiments carried out with the early synchrotron sources, from 1960 to about 1995, are reviewed, including photoionization of unpolarized and polarized excited atoms, and time-resolved laser–synchrotron studies. With the most advanced generation of synchrotron sources, a whole new class of pump–probe experiments benefiting from the high brightness of the new synchrotron beams has been developed since 1996. A detailed review of these studies as well as possible future applications of pump–probe experiments using third generation synchrotron sources and free electron lasers is presented.


PACS

32.80.Fb Photoionization of atoms and ions

32.80.Hd Auger effect (including Coster-Krönig transitions)

32.80.Xx Level crossing and optical pumping

42.55.Mv Dye lasers

41.60.Ap Synchrotron radiation

41.60.Cr Free-electron lasers

Subjects

Atomic and molecular physics

Accelerators, beams and electromagnetism

Optics, quantum optics and lasers

Dates

Issue 23 (14 December 2006)

Received 12 July 2006, in final form 6 October 2006

Published 17 November 2006



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