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Investigation of valence inter-multiplet Auger transitions in Ne following 1s photoelectron recapture

A De Fanis1, G Prümper2, U Hergenhahn2,3, E Kukk2,4, T Tanaka5, M Kitajima5, H Tanaka5, S Fritzsche6, N M Kabachnik7,8 and K Ueda2

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We employ a novel technique in which highly excited Rydberg states of Ne+ 2p4np are populated via PCI-induced recapture of the near-threshold 1s photoelectron (De Fanis et al 2004 Phys. Rev. A 70 040702) to investigate valence inter-multiplet Auger transitions. The following series of the transitions have been observed: Ne+ 2p4(1D)np 2L → Ne2+ 2p4 3PJ, Ne+ 2p4(1S)np 2P →Ne2+ 2p4 3PJ and Ne+ 2p4(1S)np 2P →Ne2+ 2p4 1D. Their energy positions, quantum defects and the anisotropy parameters of the Auger electron emission have been determined. Experimental results are in good agreement with multi-configuration Dirac–Fock calculations carried out as a part of this study. The importance of interference effects for decays via naturally overlapping fine-structure components of the intermediate state is discussed.


PACS

32.80.Hd Auger effect (including Coster-Krönig transitions)

32.80.Rm Multiphoton ionization and excitation to highly excited states

31.15.-p Calculations and mathematical techniques in atomic and molecular physics

32.80.Fb Photoionization of atoms and ions

32.10.Fn Fine and hyperfine structure

Subjects

Atomic and molecular physics

Computational physics

Dates

Issue 13 (14 July 2005)

Received 21 February 2005, in final form 4 May 2005

Published 14 June 2005



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