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High-order above-threshold multiphoton detachment of H: time-dependent non-Hermitian Floquet approach

Dmitry A Telnov1 and Shih-I Chu

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We present a nonperturbative quantum study of high-order above-threshold detachment of H in intense laser fields using an accurate one-electron model potential and a new time-dependent non-Hermitian Floquet approach. Detailed exploration of the electron energy and angular distributions is pursued for the laser field intensities 1010–1011 W cm−2 and wavelength 10.6 µm. In accordance with semiclassical predictions, the electron energy spectrum exhibits a plateau region in the higher energy part. Transformation of the electron angular distributions in the plateau region is discussed. The computational method involves the complex-scaling generalized pseudospectral (CSGPS) spatial discretization of the Hamiltonian and non-Hermitian time propagation of the time-evolution operator by means of the split-operator technique in the energy representation. The approach is designed for effective treatment of multiphoton processes in very intense and/or low-frequency laser fields, which are generally more difficult to treat using the conventional time-independent Floquet matrix techniques.


PACS

32.80.Rm Multiphoton ionization and excitation to highly excited states

31.15.E- Density-functional theory

32.80.Gc Photodetachment of atomic negative ions

Subjects

Atomic and molecular physics

Computational physics

Dates

Issue 7 (14 April 2004)

Received 27 November 2003

Published 17 March 2004



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