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Coplanar dissociation of ethylene and benzene by collision with Ar8+

G Veshapidze, M Nomura, T Nishide1, F A Rajgara2, H Shiromaru, Y Achiba and N Kobayashi

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By collision of 120 keV Ar8+ with planar hydrocarbons, ethylene and benzene, dissociation of multiply ionized target molecules was studied, focusing attention on the possibility that all the fragment ions are ejected, or tend to be ejected, in a single plane. The trajectories of fragment ions were determined by position-sensitive time-of-flight measurements and the angular correlation of the initial velocity vectors was compared to the results of a reference non-planar molecule, ethane. To eliminate ambiguity due to the contribution of the residual gases, dissociation of ethylene-d4 and benzene-d6 was also examined. The results indicate that the initial velocity direction of the fragments indeed tends to be confined in a single plane when the target molecules are planar. That is, the angular correlation of fragment ions conserves the information on the molecular structure even for considerably large molecules.


PACS

33.15.Fm Bond strengths, dissociation energies

33.15.Bh General molecular conformation and symmetry; stereochemistry

07.57.-c Infrared, submillimeter wave, microwave and radiowave instruments and equipment

Subjects

Atomic and molecular physics

Instrumentation and measurement

Dates

Issue 14 (28 July 2004)

Received 1 April 2004

Published 8 July 2004



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