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Shape-resonance-induced long-range molecular Rydberg states

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Edward L Hamilton1, Chris H Greene1 and H R Sadeghpour2

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LETTER TO THE EDITOR

When an excited atomic electron interacts with a neutral perturbing atom or molecule that possesses a shape resonance, it generates a characteristic class of Born-Oppenheimer potential curves that rise with internuclear distance. We document this effect, and predict the existence of a diverse class of stable, strongly bound atom-atom and atom-molecule states that result from this phenomenon. For the specific case in which Rb is the perturbing atom, we show that such states should be observable in the spectroscopy of an ultracold gas or condensate.


PACS

33.80.Rv Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)

37.10.Mn Slowing and cooling of molecules

37.10.De Atom cooling methods

31.15.xp Perturbation theory

32.80.Rm Multiphoton ionization and excitation to highly excited states

Subjects

Atomic and molecular physics

Computational physics

Dates

Issue 10 (28 May 2002)

Received 22 April 2002

Published 8 May 2002



  1. Shape-resonance-induced long-range molecular Rydberg states

    Edward L Hamilton et al 2002 J. Phys. B: At. Mol. Opt. Phys. 35 L199

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