A De Fanis et al 2002 J. Phys. B: At. Mol. Opt. Phys. 35 L23 doi:10.1088/0953-4075/35/1/104
Control of nuclear motion in the B 2b2 ionic state of water via an Auger resonant Raman process
FREE ARTICLEA De Fanis1, K Nobusada2, I Hjelte3, N Saito4, M Kitajima5, M Okamoto5, H Tanaka5, H Yoshida6, A Hiraya6, I Koyano7, M N Piancastelli8 and K Ueda1,9
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Resonant Auger spectra of H2O are recorded with unprecedented resolution, for excitation energies tuned across the O 1s→2b2 resonance. Electron emission spectra for decay to the 1b2-1 final state show a partially resolved vibrational envelope whose overall appearance is photon energy dependent. Comparison with ab initio calculations indicates that the two-dimensional nuclear motion of the Auger final state can be controlled by sampling different portions of the potential curve and changing the nuclear motion in the core-excited state.
- PACS
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33.80.Eh Autoionization, photoionization, and photodetachment
34.35.+a Interactions of atoms and molecules with surfaces
33.70.Jg Line and band widths, shapes, and shifts
33.20.Fb Raman and Rayleigh spectra (including optical scattering)
- Subjects
- Dates
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Issue 1 (14 January 2002)
Received 4 October 2001
Published 19 December 2001
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Control of nuclear motion in the B 2b2 ionic state of water via an Auger resonant Raman process
A De Fanis et al 2002 J. Phys. B: At. Mol. Opt. Phys. 35 L23
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