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Evidence of enhanced multiphoton (248 nm) coupling from single-pulse energy measurements of Xe(L) emission induced from Xe clusters

A McPherson-+, J Cobble++, A B Borisov-+, B D Thompson-+, F Omenetto-+, K Boyer-+ and C K Rhodes-+

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LETTER TO THE EDITOR

Single-pulse energy measurements of the Xe(L) emission induced by femtosecond multiphoton ultraviolet (248 nm) excitation of Xe clusters have been made with a transmission grating spectrograph equipped with a calibrated x-ray CCD camera. On the basis of the observed magnitude of the Xe(L) single-pulse yield and the morphology measured by Thomson scattering of the self-trapped channels guiding the incident 248 nm pulse, it is concluded that the coupling strength for x-ray production from the clusters cannot be accounted for by an interaction involving only independent single-electron processes. Analysis indicates that the coupling requires augmentation by a factor of . This conclusion is in good agreement with an independent spectral study involving the direct comparison of the multiphoton coupling strength with electron collisional data for Xe obtained from EBIT studies, an analysis which placed the corresponding factor of augmentation of the coupling in the interval . These findings are consistent with estimates of the magnitude of the strengthened coupling which could arise from the development of ordered multi-electron motions.


PACS

36.40.Mr Spectroscopy and geometrical structure of clusters

33.80.Rv Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)

33.20.Lg Ultraviolet spectra

Subjects

Atomic and molecular physics

Dates

Issue 21 (14 November 1997)

Received 7 July 1997, in final form 9 September 1997



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