Quick search Find article
Quick search
Find article

NMR relaxation rates and Knight shifts in MgB2 and AlB2: theory versus experiments

E Pavarini1, S H Baek2, B J Suh3, F Borsa1,2, S L Bud'ko2 and P C Canfield2

Show affiliations


We have performed 11B NMR measurements in 11B enriched MgB2 powder sample in the normal phase. The Knight shift was accurately determined by using the magic angle spinning technique. Results for 11B and 27Al Knight shifts (K) and relaxation rates (1/T1) are also reported for AlB2. The data show a dramatic decrease of both K and 1/T1 for 11B in AlB2 with respect to MgB2. We compare experimental results with ab initio calculated NMR relaxation rates and Knight shifts. The experimental values for 1/T1 and K are in most cases in good agreement with the theoretical results. We show that the decrease of K and 1/T1 for 11B is consistent with a drastic drop of the density of states at the boron site in AlB2 with respect to MgB2.


PACS

76.60.Cq Chemical and Knight shifts

74.25.Nf Response to electromagnetic fields (nuclear magnetic resonance, surface impedance, etc.)

74.25.Jb Electronic structure

74.70.Ad Metals; alloys and binary compounds (including A15, MgB2, etc.)

76.60.Es Relaxation effects

71.15.Mb Density functional theory, local density approximation, gradient and other corrections

Subjects

Superconductivity

Condensed matter: electrical, magnetic and optical

Dates

Issue 2 (February 2003)

Received 29 June 2002

Published 30 December 2002



View by subject




Export








Please login to access our web services, or create an account if you don't yet have one.

You must have cookies enabled in your web browser to be able to login.

Username
Password

Forgotten your password? Get a new one here.