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Measurement and modeling of hydrogen molecule ro-vibrational accommodation on E-294 polycrystalline graphite

E M Hollmann1, P S Krstic2, R P Doerner1, D Nishijima1, A Yu Pigarov1, C O Reinhold2 and S J Stuart3

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BRIEF COMMUNICATION

The loss rate of H2 and D2 internal ro-vibrational energy in collisions with an E-294 polycrystalline graphite surface is measured in a plasma-free environment. Accommodation coefficients are found to be approximately 0.01–0.2 for vibrational energy and somewhat larger, 0.05–0.2 for rotational energy, with a slight increasing trend seen with increasing surface temperature. Molecular dynamics simulations of the experiment give a total ro-vibrational accommodation rate of order 0.1, which is consistent with the data at higher surface temperatures.


PACS

52.20.Hv Atomic, molecular, ion, and heavy-particle collisions

33.20.Vq Vibration-rotation analysis

52.65.Yy Molecular dynamics methods

52.55.Fa Tokamaks, spherical tokamaks

Subjects

Atomic and molecular physics

Plasma physics

Dates

Issue 10 (October 2008)

Received 1 July 2008, in final form 10 August 2008

Published 10 September 2008



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