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Maximum entropy production and the fluctuation theorem

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R C Dewar

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LETTER TO THE EDITOR

Recently the author used an information theoretical formulation of non-equilibrium statistical mechanics (MaxEnt) to derive the fluctuation theorem (FT) concerning the probability of second law violating phase-space paths. A less rigorous argument leading to the variational principle of maximum entropy production (MEP) was also given. Here a more rigorous and general mathematical derivation of MEP from MaxEnt is presented, and the relationship between MEP and the FT is thereby clarified. Specifically, it is shown that the FT allows a general orthogonality property of maximum information entropy to be extended to entropy production itself, from which MEP then follows. The new derivation highlights MEP and the FT as generic properties of MaxEnt probability distributions involving anti-symmetric constraints, independently of any physical interpretation. Physically, MEP applies to the entropy production of those macroscopic fluxes that are free to vary under the imposed constraints, and corresponds to selection of the most probable macroscopic flux configuration. In special cases MaxEnt also leads to various upper bound transport principles. The relationship between MaxEnt and previous theories of irreversible processes due to Onsager, Prigogine and Ziegler is also clarified in the light of these results.


PACS

05.70.Ce Thermodynamic functions and equations of state

05.70.Ln Nonequilibrium and irreversible thermodynamics

02.50.Cw Probability theory

05.40.-a Fluctuation phenomena, random processes, noise, and Brownian motion

MSC

60Exx Distribution theory (See also 62Exx, 62Hxx)

82B35 Irreversible thermodynamics, including Onsager-Machlup theory (See also 92E20)

Subjects

Computational physics

Statistical physics and nonlinear systems

Dates

Issue 21 (27 May 2005)

Received 22 December 2004, in final form 13 April 2005

Published 10 May 2005



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