Strong-field ionization in time-dependent density functional theory

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Published 10 November 2008 Europhysics Letters Association
, , Citation A. S. de Wijn et al 2008 EPL 84 43001 DOI 10.1209/0295-5075/84/43001

0295-5075/84/4/43001

Abstract

Ionization in a strong laser field is a prime example of non-perturbative, correlated electron dynamics. Simulating such processes on a first-principles basis is a major theoretical challenge. We demonstrate that time-dependent density functional theory (TDDFT) on the basis of a newly developed functional for the correlation potential incorporates the relevant electron interaction effects. The central idea of our approach is to exploit information about exact ground-state correlation in approximate time-dependent calculations. The new functional provides an accurate description of the paradigm problem of the double ionization of the Helium atom, showing that TDDFT is a viable tool for strong-field calculations.

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10.1209/0295-5075/84/43001