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Magnetic ordering in the striped nickelate La5/3Sr1/3NiO4: A band structure point of view

U. Schwingenschlögl1, C. Schuster1 and R. Frésard2

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We report on a comprehensive study of the electronic and magnetic structure of the striped nickelate La5/3Sr1/3NiO4. The investigation is carried out using band structure calculations based on the density functional theory. A magnetic structure compatible with experiment is obtained from spin-polarized calculations within the generalized gradient approximation (GGA), whereas inclusion of a local Coulomb interaction in the LDA+U framework results in a different ground state. The influence of the various interaction parameters is discussed in detail.


PACS

71.45.Lr Charge-density-wave systems

75.25.+z Spin arrangements in magnetically ordered materials (including neutron and spin-polarized electron studies, synchrotron-source x-ray scattering, etc.)

71.20.-b Electron density of states and band structure of crystalline solids

Subjects

Condensed matter: electrical, magnetic and optical

Dates

Issue 2 (January 2008)

Received 20 August 2007, accepted for publication 7 November 2007

Published 4 December 2007



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