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Raman scattering study of cubic GaN and GaMnN epilayers grown by plasma- assisted molecular beam epitaxy

E Alarcón-Lladó1, J Ibáñez1, R Cuscó1, L Artús1, S V Novikov2 and C T Foxon2

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We perform visible and ultraviolet (UV) Raman-scattering experiments to study a series of undoped and Mn-doped c-GaN thin films grown by plasma-assisted molecular beam epitaxy under Ga-rich and N-rich conditions. The visible, non-resonant experiments confirm that the Ga-rich growth yields the improved crystal quality. New Raman features, most probably related to Mn-induced disorder, show up in the spectra of the c-GaMnN epilayers grown under N-rich conditions. We find that the introduction of an AlN buffer favors the growth of the hexagonal phase. In the UV spectra of the samples with better crystal quality, we detect multiphonon mA1(LO) peaks up to m = 4 together with strong PL signal from c-GaN. In the more disordered samples the PL emission is quenched, and this allows us to detect multiphonons up to m = 6. The intensity of the multiphonon peaks can be used to assess the crystal quality of the c-GaN and c-GaMnN samples.


PACS

81.15.Hi Molecular, atomic, ion, and chemical beam epitaxy

68.55.A- Nucleation and growth

78.66.Fd III-V semiconductors

78.30.Fs III-V and II-VI semiconductors

68.55.Ln Defects and impurities: doping, implantation, distribution, concentration, etc.

78.55.Cr III-V semiconductors

Subjects

Condensed matter: electrical, magnetic and optical

Semiconductors

Surfaces, interfaces and thin films

Dates

Issue 11 (November 2009)

Received 17 July 2009

Published 27 October 2009



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