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Synthesizing Metastable Rocksalt-Type MgTe Based on High-Pressure Solid-State Phase Transition: A First-Principles Study

Cai Ying-Xiang1 and Xu Rui2

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ATOMIC AND MOLECULAR PHYSICS

The controllability of pressure-induced structural transformation in the hexagonal wurtzite-type MgTe is studied by a first-principles pseudopotential method within the generalized gradient approximation (GGA). Based on the transitional mechanisms of the wurtzite→—NiAs and the wurtzite→—rocksalt, a special method of loading biaxial pressure on the (010) and (001) planes of an orthorhombic cell is designed. At equal biaxial pressure of 2.75 GPa, an abrupt volume collapse is found and the WZ phase transforms into an orthorhombic phase with a tiny distortion. While the pressure decreases to zero, three lattice parameters a, b and c become equal and a metastable rocksalt–type MgTe is obtained.


PACS

81.20.-n Methods of materials synthesis and materials processing

64.70.K- Solid–solid transitions

61.66.Fn Inorganic compounds

62.50.-p High-pressure effects in solids and liquids

Subjects

Condensed matter: structural, mechanical & thermal

Dates

Issue 11 (November 2009)

Received 3 April 2009



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