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Magnetic ordering in arrays of one-dimensional nanoparticle chains

D Serantes1, D Baldomir1, M Pereiro1, B Hernando2, V M Prida2, J L Sánchez Llamazares2, A Zhukov3, M Ilyn3 and J González3

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The magnetic order in parallel-aligned one-dimensional (1D) chains of magnetic nanoparticles is studied using a Monte Carlo technique. If the easy anisotropy axes are collinear along the chains a macroscopic mean-field approach indicates antiferromagnetic (AFM) order even when no interparticle interactions are taken into account, which evidences that a mean-field treatment is inadequate for the study of the magnetic order in these highly anisotropic systems. From the direct microscopic analysis of the evolution of the magnetic moments, we observe spontaneous intra-chain ferromagnetic (FM)-type and inter-chain AFM-type ordering at low temperatures (although not completely regular) for the easy-axes collinear case, whereas a random distribution of the anisotropy axes leads to a sort of intra-chain AFM arrangement with no inter-chain regular order. When the magnetic anisotropy is neglected a perfectly regular intra-chain FM-like order is attained. Therefore it is shown that the magnetic anisotropy, and particularly the spatial distribution of the easy axes, is a key parameter governing the magnetic ordering type of 1D-nanoparticle chains.


PACS

75.75.+a Magnetic properties of nanostructures

75.40.Mg Numerical simulation studies

75.50.Ee Antiferromagnetics

75.30.Cr Saturation moments and magnetic susceptibilities

75.30.Gw Magnetic anisotropy

75.50.Tt Fine-particle systems; nanocrystalline materials

Subjects

Condensed matter: electrical, magnetic and optical

Nanoscale science and low-D systems

Dates

Issue 21 (7 November 2009)

Received 29 July 2009, in final form 1 September 2009

Published 13 October 2009



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