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Tuning the bandgap of InAs quantum dots by selective-area MOCVD

S Mokkapati1,3, J Wong-Leung1, H H Tan1, C Jagadish1, K E McBean2 and M R Phillips2

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In-plane bandgap energy control of InAs quantum dots (QDs) grown on GaAs substrates is demonstrated using selective-area epitaxy. Transmission electron microscopy and cathodoluminescence are used for characterization of the selectively grown dots. A single-step growth of a thin InAs quantum well and InAs QDs emitting at 1010 and 1100 nm (at 77 K) on the same wafer is demonstrated. Non-uniform growth profile is reported for the selectively grown QDs in the mask openings. Surface migration of adatoms from higher order facets to (1 0 0) facets results in enhanced deposition rates closer to the edge of the openings and vapour phase diffusion of adatoms results in density variations across the openings over length scales greater than the surface migration length of the adatoms.


PACS

73.21.La Quantum dots

68.37.Lp Transmission electron microscopy (TEM)

78.60.Hk Cathodoluminescence, ionoluminescence

68.55.A- Nucleation and growth

81.15.Gh Chemical vapor deposition (including plasma-enhanced CVD, MOCVD, etc.)

68.65.Hb Quantum dots (patterned in quantum wells)

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 8 (21 April 2008)

Received 7 November 2007, in final form 4 February 2008

Published 14 March 2008



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