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Morphology transformation of patterned, uniform and faceted GaN microcrystals

Tae Woong Kim1, Young Joon Hong2, Gyu-Chul Yi2, Ji-Hwan Kwon1, Miyoung Kim1, Heung Nam Han1, Do Hyun Kim1, Kyu Hwan Oh1, Ki-jeong Kong3 and Young-Kyun Kwon4

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We report on the growth and characterization of patterned and uniformly distributed GaN microcrystals with well-defined facets and epitaxy. The microcrystals were grown on a mask patterned by lithography. The GaN microcrystals were formed by selective-area epitaxy using metal-organic chemical-vapour deposition. The GaN microcrystals have similar sizes and shapes. Each microcrystal consists of an upper and a lower part, which are rotated by 30°. Transmission electron microscopy shows that there is a rather clear interface between the two parts of the crystal, suggesting a sudden change in the growth direction. We performed ab initio calculations for the surface energies of hexagonal GaN, and the growth morphology is explained based on surface energy considerations.


PACS

68.55.-a Thin film structure and morphology

81.16.Nd Nanolithography

68.35.Md Surface thermodynamics, surface energies

64.70.Nd Structural transitions in nanoscale materials

81.15.Gh Chemical vapor deposition (including plasma-enhanced CVD, MOCVD, etc.)

Subjects

Surfaces, interfaces and thin films

Condensed matter: structural, mechanical & thermal

Nanoscale science and low-D systems

Dates

Issue 1 (7 January 2008)

Received 4 October 2007, in final form 12 November 2007

Published 19 December 2007



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