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Ultrafast decay of femtosecond laser-induced grating in silicon-quantum-dot-based optical waveguides

I Pelant1,6, R Tomašibar unas2, V Sirutkaitis3, J Valenta4, T Ostatnický4, K Kůsová1 and R G Elliman5

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Femtosecond transient laser-induced grating (LIG) experiments were performed in planar optical waveguides made of luminescent silicon quantum dots. The LIG was created by interference of two pulses from the frequency-doubled output of a Ti–sapphire laser (400 nm, 400 fs, 1 kHz). The LIG exhibits an extremely fast decay in time (several picoseconds) that was found to decrease with decreasing grating period. The standard models based on lateral carrier diffusion cannot explain this observation (this procedure yields an unrealistically high diffusion constant of 420 cm2 s−1). Instead, the results are explained by exciton diffusion and/or enhanced exciton radiative decay rate in a cavity represented by the periodically modulated planar waveguide (Purcell effect).


PACS

78.47.-p Spectroscopy of solid state dynamics

42.79.Gn Optical waveguides and couplers

78.67.Hc Quantum dots

Subjects

Condensed matter: electrical, magnetic and optical

Optics, quantum optics and lasers

Nanoscale science and low-D systems

Dates

Issue 1 (7 January 2008)

Received 17 September 2007, in final form 25 October 2007

Published 12 December 2007



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