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Electron spin resonance of europium in silver chloride

S U Cheema and M J A Smith

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Europium added to silver chloride under a nonoxidizing atmosphere enters the lattice substitutionally in the divalent state. A single silver ion vacancy is associated with each europium ion in a nearest cation position at 93 K and leads to an electron resonance which shows orthorhombic symmetry. At room temperature most of the vacancies are dissociated and the predominant spectrum arises from Eu2+ in a field of octahedral symmetry. The temperature variation in the width of lines which constitute the outer fine structure components of the spectrum gives an activation energy of 0.22+or-0.05 eV for the vacancy motion. In heavily doped specimens a single line spectrum is observed from aggregated europium. Eu2+ is found to sensitize silver chloride in the bulk. At room temperature irradiation with blue light produces a reduction in the number of Eu2+ ions and an optical absorption peak at 550 nm due to silver colloid, Irradiation with red light bleaches the colloid band and restores the original number of Eu2+ ions.


PACS

76.30.Kg Rare-earth ions and impurities

61.72.J- Point defects and defect clusters

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 10 (30 July 1971)



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